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研究生:洪鴻斌
研究生(外文):Hung, Hung-Ping
論文名稱:使用H2O2/UV和H2O2/UV/Fe2+程序處理難分解染料製程廢水
論文名稱(外文):Treatment of Refractory Dyestuffs Wastewater Using H2O2/UV和H2O2/UV/Fe2+ Processes
指導教授:康世芳康世芳引用關係
指導教授(外文):Kang, Shyh-Fang
學位類別:碩士
校院名稱:淡江大學
系所名稱:水資源及環境工程學系
學門:工程學門
學類:環境工程學類
論文種類:學術論文
論文出版年:1997
畢業學年度:85
語文別:中文
論文頁數:106
中文關鍵詞:染料H2O2/UV和H2O2/UV/Fe2+程序
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本研究在探討染料製程之實廠廢水,使用高級氧化H2O2/UV與H2O2/UV/Fe2+兩程序作為前處理來減輕後續處理單元之負荷,及了解反應程序進行之重要機制,有助於最佳程序之設計。染料製程廢水具有高濃度之難分解有機物、色度濃厚及無機鹽類(如Cl-或SO42-)含量高,若未經妥善處理,對承受水體水質將造成極嚴重的威脅。由國內外文獻回顧得知,染料成份對生物具有抑制作用,目前大都無法單獨使用生物處理去除,需搭配使用其它各種高級氧化程序(Advanced Oxidation Processes 簡稱AOPs)。以H2o2/UV程序及配合添加亞鐵探討其處理染料製程實廠廢水之成效,此二程序皆可產生具強氧化能力的氫氧自由基(OH.),能有效地氧化目標污染物有機成份,由此探討操作參數(H2O2、Fe2+劑量、UV強度)及水質參數(pH值、氯離子濃度、廢水強度)對程序效率之影響。
根據實驗結果得知,添加過量的H2O2劑量對COD之去除於兩種程序中並無顯著的提昇,至於ABS254與ADMI的去除速率則比COD來的快。去除ABS254與用ADMI以pH=4最佳,COD以pH=3最佳。溶液中若有氯離子存在,對COD、ABS254與ADMI等之去除產生抑制作用,唯H2O2對之裂解,在較高濃度的Cl-之情況下,影響不大。H2O2/UV與H2O2/UV/Fe2+兩程序對目標污染物的去除速率,前者之反應速率遠低於後者,但最終之去除效率兩者差異不大。建議於H2O2/UV/F2+"程序之實際操作時,在反應前期加入適量的Fe2+,配合後期補充適量之H2O2,以達到最佳程序處理效率。
This study was conducted to treat dye manufacturing wastewater using H2O1/UV and H2O2/UV/Fe2+ processes, which serve to pretreat the loading in the subsequent treatment processes or polish the secondary effluent to comply with discharge regulation. Dye manufacturing wastewater, if not appropriately treated, might impose on the receiving waters a severe threat because of its high levels of refractory organic compounds, color, and chloride ion salt. Base on the literature report, it is understood that dyestuff can not be completely removed by biological treatment, due to its inhibiting effect microorganism. Both processes mentioned above are capable of generating strong oxidant, called hydroxyl radical, which can oxidize effectively the target organics to achieve the treatment goal. The emphasis of this study was placed on the effect of ferrous ions and peroxide dosages, UV intensity, chloride ions concentration, pH, and dilution ratio of original wastewater sample on the residual fractions of COD, H2O2, ABS254 and ADMI color value. As a result the enhanced effect by adding excess H2O2 is very limited due to its OH‧ scavenging. In general, the removals of ABS254, ADMI color value were found faster than that of COD. The pH condition for the best removal of ABS254, ADMI color value, and COD occurs at around pH=3 or pH=4. Chloride ions show some inhibiting in removing COD, ABS254 and ADMI color value, however, its inhibiting effect on peroxide decomposition dose not necessarily increase with its concentration. Although, both processes show the some removal efficiency at the end of 2 hour reaction period, the removal rate is much slower using H2O2/UV process than H2O2/UV/Fe2+ process. It is suggested that add appropriate ferrous dosage in the early reaction period and then followed by supplementing sufficient amount H2O2 in the late reaction, in order to achieve the best process performance.
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