參考文獻
1.何國川,“電化學與無窗簾時代”,化工,第37卷,第3期,1990年,32-41頁。
2.焦小浣、胡文玲、陳玲,“光窗透明材料的實驗研究”,太陽能學報,第8卷,第4期,1997年,365-370頁。
3.S.E. Selkowitz and C.M. Lampert, “Large-area chromogenics: materials and devices for transmittance control”, SPIE, (1988) 22-45.
4.C.G. Granqvist, E. Avendano and A. Azens, “Electrochromic coatings and devices: Survey of some recent advances”, Thin Solid Films, 442 (2003) 201-211.
5.C.G. Granqvist, A. Azens, P. Heszler, L.B. Kish and L.O. sterlund, “Nanomaterials for benign indoor environments: electrochromics for smart windows air cleaning”, Solar Energy Materials & Solar Cells, 91 (2007) 355-365.
6.http://www.sage-ec.com/pages/projgallery_res.html
7.http://big5.nikkeibp.com.cn/news/auto/18186-200501120109.html?isRedirected=1
8.F. Carpi and D. De Rossi, “Colours from electroactive polymers: Electrochromic, electroluminescent and laser devices based on organic materials”, Optics and Laser Technology, 38 (2006) 292-305.
9.H. Pettersson, T. Gruszecki, L.H. Johansson, M.O.M. Edwards, A. Hagfeldt and T. Matuszczyk, “Direct-driven electrochromic displays based on nanocrystalline electrodes”, Displays, 25 (2004) 223-230.
10.G.G. Barna, “Material and device properties of a solid state electrochromic display”, Journal of Electronic Materials, 8 (1979) 153-173.
11.J.R. Platt, “Electrochromism: a possible change of color producible in dyes by an electric field”, Journal of Chemical Physics, 34 (1961) 862-863.
12.林保彰,“三氧化鎢薄膜電極之製備及其電致色變性質之研究”,國立台灣大學化學工程學研究所碩士論文,1998。
13.M.A. Habib and D. Glueck, “The electrochromic properties of chemically deposited tungsten oxide films”, Solar Energy Materials, 18 (1989) 127-141.
14.T. Yoshino, N. Baba, H. Masuda and K. Arai, “A new method for preparing electrochromic IrOχ thin films by periodic reverse electrolysis of sulfatoiridate complex”, The Electrochemical Society Softbound Proceedings Series, 90-2 (1990) 89-98.
15.P. Pfluger, H.U. Künzi and H.J. Güntherodt, “Discovery of a new reversible electrochromic effect”, Applied Physics Letter, 35 (1979) 771-772.
16.J. Nagao, “Characterization of evaporated nickel oxide and its application to electrochromic glazing”, Solar Energy Materials and Solar Cells, 31 (1993) 291-299.
17.S. Gottesfeld, “The anodic rhodium oxide film-a two-color electrochromic system”, Journal of the Electrochemical Society, 127 (1980) 272-277.
18.K. Boufker, “Lithiation study of molybdenum oxide thin-films- application to an electrochromic system”, Journal of Applied Electrochemistry, 25 (1995) 797-802.
19.C.K. Dyer and J.S.L. Leach, “Reversible optical changes within anodic oxide films on titanium and niobium”, Journal of the Electrochemical Society, 125 (1978) 23-29.
20.T. Ohtasuka, M. Masuda and N. Sato, “Cathodic reduction of anodic oxide films formed on titanium”, Journal of the Electrochemical Society, 134 (1987) 2406-2410.
21.K. Itaya, K. Shibayama, H. Akahshi and S. Toshima, “Prussian-blue- modified electrodes: an application for a stable electrochromic display device”, Journal of Applied Physics, 53 (1982) 804-805.
22.D.D. Deford and A.W. Davidson, “Studies on the oxidation of potassium ruthenocyanide”, Journal of the American Chemical Society, 73 (1951) 1469-1474.
23.Z. Gao, G. Wang, P. Li and Z. Zhao, “Electrochemical and spectroscopic studies of cobalt-hexacyanoferrate film modified electrodes”, Electrochimica Acta, 36 (1991) 147-152.
24.D. Shaojun and L. Fengbin, “Researches on chemically modified electrodes: Part XV. preparation and electrochromism of the vanadium hexacyanoferrate film modified electrode”, Journal of Electroanalytical Chemistry, 210 (1986) 31-44.
25.K.J. Kulesza and M. Faszynska, “Indium (III)-hexacyan of errate as a novel polynuclear mixed-valent inorganic material for preparation of thin zeolitic films on conducting substrates”, Journal of Electroanalytical Chemistry, 252 (1988) 461-466.
26.R.V. Pole, G.T. Sincerbox and M.D. Shattuck, “Photoinduced electrochromic effect and its applications to displays”, Applied Physics Letters, 28 (1976) 494-497.
27.N.R. Lynam and A.Agrawal, “Large-area chromogenic: materials and devices for transmittance control”, SPIE Optics Engineering Press, 4 (1990) 335-365.
28.F.B. Kaufman, E.M. Engler, V.V. Patel and A.H. Schroeder, “Polymer-modified electrodes : a new class of electrochromic materials”, Applied Physics Letters, 36-6 (1979) 422-425.
29.S.K. Deb, “A novel electrophotographic systems”, Applied Optics, 3 (1969) 192.
30.F.G.K. Baucke, “Electrochromic applications”, Materials Science and Engineering B, 10 (1991) 285-292.
31.D.J. You, S.K. Choi, H.S. Han, J.S. Lee and C.B. Lim, “Effect of the deposition geometry on the electrical properties within tin-doped indium oxide film deposited under a given RF magnetron sputtering condition”, Thin Solid Films, 401 (2001) 229-234.
32.C.M. Lampert, “Smart switchable glazing for solar energy and daylight control”, Solar Energy Materials and Solar Cells, 52 (1998) 207-221.
33.G. Leftheriotis, S. Papaefthimiou, P. Yianoulis and A. Siokou, “Effect of the tungsten oxidation states in the thermal coloration and bleaching of amorphous WO3 films”, Thin Solid Films, 384 (2001) 298-306.
34.A. Donnadieu, “Electrochromic materials”, Material Science and Engineering B, 3 (1989) 185-195.
35.S.J. Babinec, “A quartz crystal microbalance analysis of ion insertion into WO3”, Solar Energy Material Solar Cells, 25 (1992) 269-291.
36.M. Kitao and S. Yamada, “Proceedings of the international seminar in solid state ionic devices”, Radhakrishna World Publishing Co., Singapore, (1988) 139.
37.M. Green, D.C. Smith and J. A. Weiner, “A thin film electrochromic display based on the tungsten bronzes”, Thin Solid Films, 38 (1976) 89-100.
38.R.B. Goldner, P. Norton, K. Wong, G. Foley, E.L. Goldner, G. Seward and R. Chapman, “Further evidence for free electrons as dominating the behavior of electrochromic polycrystalline WO3 films”, Applied Physics Letters, 47 (1985) 536-538.
39.G.G. Barna, “Material and device properties of a solid state electrochromic display”, Journal of Electronic Materials, 8 (1979) 153-173.
40.S.J. Babinec, “A quartz crystal microbalance analysis of ion insertion into WO3”, Solar Energy Material Solar Cells, 25 (1992) 269-291.
41.B. Reichman and A. J. Bard, “The electrochromic process at WO3 electrodes prepared by vacuum evaporation and anodic oxidation of WO3”, Journal of The Electrochemical Society, 126 (1979) 583-591.
42.S. K. Deb, “Optical and photoelectric properties and colour centres in thin films of tungsten oxide”, Philosophical Magazine, 27 (1973) 801-822.
43.A. Deneuville, P. Gerard and R. Billat, “Principles and operation of an all solid state electrochromic display based on a-‘WO3’ ”, Thin Solid Films, 70 (1980) 203-223.
44.F. Beck and M. Dahlhaus, “Anodic formation of polypyrrole tungsten trioxide composites”, Journal of Applied Electrochemistry, 23 (1993) 781-789.
45.M. Dahlhaus and F. Beck, “Characterization of anodically formed polypyrrole tungsten trioxide composites”, Journal of Applied Electrochemistry, 23 (1993) 957-965.
46.L.L. Hensch and J.K. West, “The sol-gel process”, Chemical Reviews 90 (1990) 33-72.
47.L.M. Schiavone, W.C. Dautremont-Smith, G. Beni and J.L. Shay, “Improved electrochromic behavior of reactively sputtered iridium oxide films”, Journal of the Electrochemical Society, 128 (1981) 1339-1342.
48.A. Maccari, G. Macrelli, P. Polato and E. Poli, “Design, production and characterization of an all solid state electrochromic medium size device”, Solar Energy, 63 (1998) 217-229.
49.P.M.S. Monk, R.J. Mortimer and D.R. Rosseinsky, “Electrochromism: fundaments and applications”, VCH, Weinheim, (1995) 45-46.
50.S.R. Jiang, P.X. Yan, B.X. Feng, X.M. Cai and J. Wang, “The response of a NiOx thin film to a step potential and its electrochromic mechanism”, Materials Chemistry and Physics, 77 (2002) 384-389.
51.A. Pennisi and F. Simone, “Electrochromic device based on tungsten- oxide and on nafion-H as polymeric electrolyte”, Applied Physics A, 57 (1993) 13-17.
52.A. Pennisi and F. Simone, “Characterization and performances of WO3:Mo/Nafion-HTM electrochromic device”, Proceedings of the Society of Photo-Optical Instrumentation Engineers, 2255 (1994) 406-414.
53.A. Pennisi and F. Simone, “An eectrochromic device working in absence of ion storage counterelectrode”, Solar Energy Materials and Solar Cells, 39 (1995) 333-340.
54.K.C. Ho, T.G. Rukavina and C.B. Greenberg, “Tungsten-oxide prussian blue electrochromic system based on a proton-conducting polymer electrolyte”, Journal of the Electrochemical Society, 141 (1994) 2061- 2067.
55.K.C. Ho, T.G. Rukavina and C.B. Greenberg, “Proceedings of the symposium on elrctrochromic materials II”, The Electrochemical Society, 94-2 (1994) 278-289.
56.K.H. Heckner and A. Rothe, “Intercalation mechanisms and time dependencies of work parameters of electrochromic layers”, Proceedings of the Society of Photo-Optical Instrumentation Engineers, 2255 (1994) 305-313.
57.M. Antinucci and A. Ferriolo, “Development of fast-response electrochromic devices on polymeric substrate”, Proceedings of the Society of Photo-Optical Instrumentation Engineers, 2255 (1994) 395-403.
58.M. Antinucci, B. Chevalier and A. Ferriolo, “Development and characterisation of electrochromic devices on polymeric substrates”, Solar Energy Materials and Solar Cells, 39 (1995) 271-287.
59.F. Michalak and P. Aldebert, “A flexible electrochromic device based on colloidal tungsten-oxide and polyaniline”, Solid State Ionics, 85 (1996) 265-272.
60.J.G. Zhang, D.K. Benson, C.E. Tracy, S.K. Deb, A.W. Czanderna and R.S. Crandall, “Optimization study of solid-state electrochromic devices based on WO3/lithium-polymer electrolyte/V2O5 structures”, Journal of the Electrochemical Society, 141 (1994) 2795-2800.
61.S. Passerini, A.L. Tipton and W.H. Smyrl, “Spin coated V2O5 XRG as optically passive electrode in laminated electrochromic devices”, Solar Energy Materials and Solar Cells, 39 (1995) 167-177.
62.P. Schlotter, G. Baur, R. Schmidt and U. Weinberg, “Laminated electrochromic device for smart windows”, Proceedings of the Society of Photo-Optical Instrumentation Engineers, 2255 (1994) 351-362.
63.B. Munro, S. Kramer, P. Zapp, H. Krug and H. Schmidt, “All sol-gel electrochromic system for plate glass”, Journal of Non-Crystalline Solids, 218 (1997) 185-188.
64.B. Munro, P. Conrad, S. Kramer, H. Schmidt and P. Zapp, “Development of electrochromic cells by the sol-gel process”, Solar Energy Materials and Solar Cell, 54 (1998) 131-137.
65.H. Inaba, M. Iwaku, K. Nakase, H. Yasukawa, I. Seo and N. Oyama, “Electrochromic display device of tungsten trioxide and prussian-blue films using polymer gel electrolyte of methacrylate”, Electrochimical Acta, 40 (1995) 227-232.
66.R. Lechner and L.K. Thomas, “All solid state electrochromic devices on glass and polymeric foils”, Solar Energy Materials and Solar Cells, 54 (1998) 139-146.
67.S.H. Lee and S.K. Joo, “Electrochromic behavior of Ni-W oxide electrodes”, Solar Energy Materials and Solar Cells, 39 (1995) 155-166.
68.B. Orel, U.O. Krasovec and U.L. Stangar, “All sol-gel electrochromic devices with Li+ ionic conductor, WO3 electrochromic films and SnO2 counter-electrode films”, Journal of Sol-Gel Science and Technology, 11 (1998) 87-104.
69.M.A. Depaoli, A. Zaneli, M. Mastragostino and A.M. Rocco, “An electrochromic device combining polypyrrole and WO3 II: solid-state device with polymeric electrolyte”, Journal of Electroanalytical Chemistry, 435 (1997) 217-224.
70.K.S. Ahn, Y.C. Nah and Y.E. Sung , “Effect of interfacial property on electrochromic response speed of Ta2O5/NiO and Ta2O5/Ni(OH)2”, Solid State Ionics, 165 (2003) 155-160.
71.Y.C. Nah, K.S. Ahn, K.Y. Cho, J.Y. Park, H.S. Shim, Y. M. Lee, J.K. Park and Y.E. Sung, “Polymer-laminated electrochromic devices composed of WO3 and Ni(OH)2 on glass and PET substrates”, Journal of the Electrochemical Society, 152 (2005) 201-204.
72.K. Kuwabara and M. Yamada , “Early cycling processes in a variable transparency ECD utilizing antimony hydrogen phosphate thin-film electrolyte”, Solid State Ionics, 59 (1993) 25-31.
73.A. Lusis , Proc. Soc. Photo-Opt. Instr. Eng. 2968(1996)167.
74.M.A. Macedo, M.A. Aegerter, “Sol-gel electrochromic device”, Journal of Sol-Gel Science and Technology, 2 (1994) 667-671.
75.A. Azens, L. Kullman, G. Vaivars, H. Nordborg and C.G. Granqvist, “Sputter-deposite nickel oxide electrochromic applications”, Solid State Ionics, 113-115 (1998 ) 449-456.
76.P.V. Ashrit, K. Benaissa, G. Bader, F.E. Girouard and V.V. Truong, “Lithiation studies on some transition-metal oxides for an all-solid thin-film electrochromic system”, Solid State Ionics, 59 (1993) 47-57.
77.N.A. O''Brien, J. Gordon, H. Mathew and B.P. Hichwa, “Electrochromic coatings- applications and manufacturing issues”, Thin Solid Films, 345 (1999) 312-318.
78.H. Yoshimura and N. Koshidaa, “Fast electrochromic effect obtained from solid-state inorganic thin-film configuration with a carrier accumulation structure”, Applied Physics Letters, 88, 093509 (2006) 1-3.
79.A. Subrahmanyam, C.S. Kumar and K.M. Karuppasamy, “A note on fast protonic solid state electrochromic device: NiOχ/Ta2O5/WO3-χ”, Solar Energy Materials and Solar Cells, 91 (2007) 62-66.
80.M. Pourbaix, “Atlas of electrochemical equilibria in aqueous solutions”, National Association of Corrous, (1974) 56-60.
81.K.S. Ahn, Y.C. Nah and Y.E. Sung, “All-solid-state electrochromic device composed of WO3 and Ni(OH)2 with a Ta2O5 protective layer”, Applied Physics Letters, 81 (2002) 3930-3932.
82.P.V. Ashrit, K. Benaissa, G. Bader, F.E. Girouard and V.V. Truong, “Lithiation studies on some transition-metal oxides for an all-solid thin-film electrochromic system”, Solid State Ionics, 59 (1993) 47-57.
83.H.L. Tuller, D.P. Button and D.R. Uhlmann, “Fast ion transport in oxide glasses”, Journal of Non-Crystalline Solids, 40 (1980) 93-118.
84.G.B. Smith, G.A. Niklasson, J.S.E.M. Svenson and C.G. Granqvist, “Noble-metal-based transparent infrared reflectors: experiments and theoretical analyses for very thin gold films”, Journal of Applied Physics, 59 (1986) 571-581.
85.A. Talledo and C.G. Granqvist, “Electrochromic vanadium- pentoxide- based films: structural, electochemical, and optical properties”, Journal of Applied Physics, 77 (1995) 4655-4666.
86.V. Eyert and K.H. Hock, “Electronic-structure of FeS2 - the crucial role of electron-lattice interaction”, Physical Review B, 57 (1998) 6350-6359.
87.P.V. Ashrit, F.E. Girouard and V.V. Truong, “Fabrication and testing of an all-solid-state system for smart window application”, Solid State Ionics, 89 (1996) 65-73.
88.I. Hamberg and C.G. Granqvist, “Color properties of transparent-ent and heat-reflecting MgF2-coated indium-tin-oxide films”, Applied Optics, 22 (1983) 609-614.
89.I. Hamberg and C.G. Granqvist, “Evaporated Sn-doped In2O3 films: basic optical properties and applications to energy-efficient windows”, Journal of Applied Physics, 60 (1986) R123-R159.
90.S.F. Cogan, R.D. Rauh, J.D. Klein, N.M. Nguyen, R.B.Jones and T.D. Plante , “Variable transmittance coatings using electrochromic lithium chromate and amorphous WO3 thin films”, Journal of the electrochemical society, 144 (1997) 956-960.
91.S.F. Cogan, R.D. Rauh, J.D. Klein, N.M. Nguyen, R.B. Jones and T.D. Plante, “Variable transmittance coatings using electrochromic lithium chromate and amorphous WO3 thin-films”, Journal of the Electrochemical Society, 144 (1997) 956-960.
92.J. Chen, Z. Zhu, Y. Zhou, R. Wang and Y. Yan, “All solid state electrochromic device: WO3/LiAlF4:Li/VO2”, Proceedings of the Society of Photo-Optical Instrumentation Engineers, 2531 (1995) 161-165.
93.A. R. Lusis, J. J. Kleperis, A. A. Brishka and E. V. Pentyush , “Electro-optic spectroscopy of electrochromic processes in tungsten trioxide”, Solid State Ionics, 13 (1984) 319-324.
94.J.G.H. Mathew, S.P. Sapers, M.J. Cumbo, N.A. O’Brien, R.B. Sargent, V.P. Raksha, R.B. Lahaderne and B.P. Hichwa, “Large area electrochromics for architectural applications”, Journal of Non-Crystalline Solids, 218 (1997) 342-346.
95.A. Daneo, G. Macrelli, P. Polato and E. Poli, “Photometric characterization of an all solid state inorganic electrochromic large area device”, Solar Energy Materials and Solar Cells, 56 (1999) 237-248
96.J. Nagai, G.D. McMeeking and Y. Saitoh, “Durability of electrochromic glazing”, Solar Energy Materials and Solar Cells, 56 (1999) 309-319.
97.C. Corbella, M. Vives, A. Pinyol, I. Porqueras, C. Person, E. Bertran, “RF sputtering deposition of Ag/ITO coatings at room temperature”, Solid State Ionics, 165 (2003) 139-148.
98.S.J. Yoo, J.W. Lim and Y.E. Sung, “Improved electrochromic devices with an inorganic solid electrolyte protective layer”, Solar Energy Materials and Solar Cells, 90 (2006) 477-484.
99.H. Yang, C. Wang, X. Diao, H. Wang, T. Wang and K. Zhu “A new all-thin-film electrochromic device using LiBSO as the ion conducting layer”, Journal of Physics D: Applied Physics, 41 (2008) 115301.
100.R.B. Goldner, F.O. Arntz and T.E. Haas, “d-Electrons and two active thin film devices for achieving a solar energy economy”, Solar Energy Materials and Solar Cells, 32 (1994) 421-428.
101.R.B. Goldner, F.O. Arntz, K. Dickson, M.A. Goldner, T.E. Haas, T. Y. Liu, S. Slaven, G. Wei, K.K. Wong and P. Zerigian, “Some lessons learned from research on a thin-film electrochromic window”, Solid State Ionics, 70-71(1994) 613-618.
102.R.B. Goldner, F.O. Arntz, K.Dickson, M.A. Goldner, T.E. Haas, T. Y. Liu, S. Slaven, G. Wei, K.K. Wong, P. Zerigian and K.C. Ho, “Proceedings of the symposium on electrochromic materials II”, The Electrochemical Society, 94-2 (1994) 237-243.
103.N. Ozer, C.M. Lampert, “Electrochrmical lithium insertion in sol-gel deposited LiNbO3 film”, Solar Energy Materials and Solar, 39 (1995) 367-375.
104.L.Q. Nguyen and V.V. Truong, “Thin film of lithium niobium oxynitride as ionic conductor”, American Institute of Physics, 80 (1996) 2914-2917.
105.X.P. Zhang, “Study on LiNbO ion conducting thin film used in electrochromic devices,” Acta Optica Sinica, 18 (1998) 803-807.
106.X. Zhang, H. Zhang, Q. Li and H. Luo, “An all-solid-state inorganic electrochromic display of WO3 and NiO films with LiNbO3 ion conductor”, IEEE Electronic Device Letters, 21 (2000) 215-217.
107.http://www.metalprices.com/FreeSite/metals/ta/ta.asp
108.J.L. He and M.C. Chiu, “Effect of oxygen on the electrochromism of RF reactive magnetron sputter deposited tungsten oxide”, Surface and Coatings Technology, 127 (2000) 43-51.
109.林郁斌、葉佳明、何紹誌、唐謙仁、何主亮,“濺鍍氧化鈮薄膜應用於電致色變元件之固態電解質層”,台灣鍍膜科技協會年會(AMTACT 2008)暨國科會專題計畫成果發表會,A01永續能源相關薄膜(Coatings for sustainable energy),論文編號02073,頁碼B54-1~4,2008年12月5-6日,彰化明道大學。
110.R. Swanepoel, “Determining refractive index and thickness of thin films from wavelength measurements only”, Journal of the Optical Society of America A-Optics Image Science and Vision, 2 (1985).
111.S.M. Rossnagel, Handbook of Plasma Processing Technology, Noyes Publications, Park Ridge, New Jersey, U.S.A, (1982) 77-88.
112.楊錦章,“基礎濺鍍電流”,電子發展月刊,第68卷,1983年,第13-40頁。
113.H. Wang, H. Shen, D. Ba, B. Wang, L. Wen, “Influence of oxygen flow on optical property of TiO2 thin film prepared by DC reactive magnetron sputtering ”, Acta Scientiarum Naturalium Unviversitatis Sunyatsen, 6 (2005) 36-40.
114.林宗隆,“¬氧化鎢、氧化鈦單層膜及多層膜知製備及其電致色變特性研究”,國立東華大學材料科學與工程研究所碩士論文,2003。
115.張智傑,“濺鍍氧化鉭薄膜應用於電致色變元件之離子傳導層研究”,逢甲大學材料科學系碩士論文,2005。116.H. Habazali, M. Yamasaki, T. Ogasawara, K. Fushimi, H. Konno, K. Shimizu, T. Izumi, R. Matsuoka, P. Skeldon and G.E. Thompson, “Thermal degradation of anodic niobia on niobium and oxygen-containing niobium”, Thin Solid Films, 516 (2008) 991-998.
117.P. Singh, B.J. Brandenburg, C.P. Sebastian, D. Kumar and O. Parkash, “XPS and mossbauer studies on BaSn1-xNbxO3(x≦0.100)”, Materials Research Bulletin, 43 (2008) 2078-2084.
118.S.A. O’Neill, I.P. Parkin, R.J.H. Clark, A. Mills and N. Elliott, “Atmospheric pressure chemical vapour deposition of thin films of Nb2O5 on glass”, Journal of Materials Chemistry, 13 (2003) 2952-2956.
119.H. Wang and C. Xie, “The effect of oxygen partial pressure on the microstructures and photocatalytic property of ZnO nanoparticles”, Physica E, 40 (2008) 2724-2729.
120.B.G. Choi, I.H. Kim, D.H Kim, K.S. Lee, T.S. Lee, B. Cheonga, Y.J. Baik and W.M. Kim, “Electrical, optical and structural properties of transparent and conducting ZnO thin films doped with Al and F by rf magnetron sputter”, Journal of the European Cearamic Society, 25 (2005) 2161-2165.
121.張智傑、何主亮、陳克昌,“應用於電致色變之濺鍍氧化鉭薄膜的鋰離子傳導能力”,中華民國防蝕工程學會94年年會論文集,第1120~1129頁,2005年8月25、26日,台灣台中。
122.余宣毅,“以RF 磁控濺鍍沉積AZO 透明導電膜之研究”,大同大學材料工程學系碩士論文,2005。