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研究生:譚莉翎
研究生(外文):Tam, Lee-Ling
論文名稱:可置換電極式III-V太陽能電池水分解研究
論文名稱(外文):Water splitting using III-V solar cell with replaceable electrodes
指導教授:洪瑞華
學位類別:碩士
校院名稱:國立交通大學
系所名稱:電子研究所
學門:工程學門
學類:電資工程學類
論文種類:學術論文
論文出版年:2019
畢業學年度:108
語文別:英文
論文頁數:41
中文關鍵詞:太陽能水分解
外文關鍵詞:Solar water splitting
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Table of content
摘要 ............................................................................................................................................... i
ABSTRACT ................................................................................................................................... ii
Acknowledgement ........................................................................................................................ iii
List of tables ................................................................................................................................... v
List of figures ................................................................................................................................. v
Chapter 1 Introduction .................................................................................................................. 1
1.1 Background ....................................................................................................................... 1
1.2 Motivation .......................................................................................................................... 2
1.3 Purpose............................................................................................................................... 2
1.4 Literature review .............................................................................................................. 3
Chapter 2 Principles ...................................................................................................................... 6
2.1 Water splitting ................................................................................................................... 6
2.2 Multi-junction III-V solar cell ......................................................................................... 7
2.3 Whole solar water splitting system .................................................................................. 7
Chapter 3 Experiments .................................................................................................................. 8
3.1 Solar cells fabrication ....................................................................................................... 8
3.2 NiFeOOH deposition ...................................................................................................... 10
3.3 Mo micro structure ......................................................................................................... 11
3.4 n-InGaN nanorods fabrication ...................................................................................... 12
3.5 Set up for OER measurement ........................................................................................ 13
3.6 Set up for solar water splitting measurement............................................................... 14
3.7 Set up for gas collection .................................................................................................. 16
Chapter 4 Results and Discussion ............................................................................................... 17
4.1 Unassisted solar water splitting ..................................................................................... 17
4.2 OER performance under different dark anode............................................................ 18
4.3 Water splitting performance in Au and NiFeOOH/Ni as dark anode ....................... 20
4.4 Mo as dark anode ............................................................................................................ 28
v
4.5 n-InGaN as dark anode .................................................................................................. 33
4.6 Difference between one and two solar cells in water splitting .................................... 35
4.7 Gas collection ................................................................................................................... 37
Reference .................................................................................................................................... 38
Chapter 5 Conclusion and Future Works .................................................................................... 40
5.1 Conclusion ....................................................................................................................... 40
5.2 Future Works .................................................................................................................. 41
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2. U.S. Department of Energy, “Hydrogen Production and Distribution,” Available: https://afdc.energy.gov/fuels/hydrogen_production.html
3. W.H. Cheng et al, “Monolithic Photoelectrochemical Device for Direct Water Splitting with 19% Efficiency,” ACS Energy Letters, vol.3, p. 1795-1800, June 2018, Available: 10.1021/acsenergylett.8b00920
4. W.H. Cheng et al, “Supporting Information for: Monolithic Photoelectrochemical Device for DirectWater Splitting with 19% Efficiency”, ACS Energy Letters, Available: https://pubs.acs.org/doi/suppl/10.1021/acsenergylett.8b00920/suppl_file/nz8b00920_si_001.pdf
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6. M. Ebaid et al, “Unbiased Photocatalytic Hydrogen Generation from Pure Water on Stable Ir-treated In0.33Ga0.67N Nanorods,” Nano Energy,2017 Available: http://dx.doi.org/10.1016/j.nanoen.2017.05.013
7. G. Peharz et al, “Solar hydrogen production by water splitting with a conversion efficiency of 18%,” Int. J. Hydrogen Energy. vol 32, p. 3248-3252, 2007, Available: https://doi.org/10.1016/j.ijhydene.2007.04.036
8. K. Sun et al, “A stabilized, intrinsically safe, 10% efficient, solar- driven water-splitting cell incorporating earth-abundant electrocatalysts with steady-state pH gradients and product separation enabled by a bipolar membrane,” Adv. Energy Matter. vol 6, 1600379 ,2016, Available: https://doi.org/10.1002/aenm.201600379
9. K. B. Oldham and J. C. Myland, Fundamentals of Electrochemical Science, Academic Press,San Diego, 1994, p. 129
10. M.M. May et al, “Efficient direct solar-to-hydrogen conversion by in situ interface transformation of a tandemstructure,” Nature Communication, Sept 2015, Available: 10.1038/ncomms9286
11. F.Dimroth et al, “Metamorphic GayIn1-yP/Ga1-xInxAs tandem solar cells for space and for terrestrial concentrator applications at C >1000 suns,” Prog. Photovolt. Res. Appl,vol 9,p 165–178,2001
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12. Y.C.Kao et al, “Performance enhancement of III–V multi-junction solar cells using indium-tin-oxide electrodes,” Thin Solid Films, May 2016, Available: http://dx.doi.org/10.1016/j.tsf.2016.05.045
13. M. Pourbaix, Atlas of Electrochemical Equilibria in Aqueous Solutions, National Association of Corrosion Engineers, Houston, 1974
14. M. Tariq et al, “Unraveling the Beneficial Electrochemistry of IrO2/MoO3 Hybrid as a Highly Stable and Efficient Oxygen Evolution Reaction Catalyst”, ACS Sustainable Chem Eng, 2018, Available: http://dx.doi.org/10.1021/acssuschemeng.7b04266
15. F.Rong et al, “Nanostructured hybrid NiFeOOH/CNT electrocatalysts for oxygen evolution reaction with low overpotential,” RSC Adv, 2016, Available: 10.1039/c6ra16450a
16. G. Park et al, “Preparation and phase transition of FeOOH nanorods: strain effects on catalytic water oxidation,” Nanoscale, 2017, Available:10.1039/c6nr09790a
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